Do you have any goals? Any limitations? Do you off-road? Is this strictly fer pavement use? Do you use the rear hatch? Which model/trim level do you have? Have you tried any mods yet? Cardboard works well fer experimentation...
Post up actual piccies of yer Jeep...
Grill block would be a start to find out how much you can block and still stay safe fer cooling. Use a digital meat thermometer to monitor under the hood temps along with an Ultragauge to monitor yer actual coolant temps. Belly pan would work. I made the one on my truck very modular and in 3 sections.
Under belly pan... - Toyota Nation Forum : Toyota Car and Truck Forums
Here's a mesh grille...so a block would be possible from behind the grill...
1999 Jeep Grand Cherokee Mesh Grille N/A
Here's what someone did to their Grand Cherokee Laredo...