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I run stock tire pressure. I know I could increase it a little, but I am too scared of the possible ill-handling effects.
It might be hard to find aftermarket sprockets for your old bike, but you never know. Cafe racer websites might be a source. As already stated, gearing is the first step. Sounds like you are all over it already.
I find that coasting is nearly impossible on a bike compared to a car. Annoyingly so, and there's not much you can do about it.
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