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There is a guy on YouTube that has many videos showing how to make car parts from fiberglass and he branched into carbon fiber and Kevlar. He says that before you make a mold, to use spackle, used to fill holes in drywall, to smooth it as much as possible. You are supposed to use Bondo, or body filler, but since you are just making a mold, you might as well save money.
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